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His murderous megalomania aside, Loki is quite charming. Just don't mention his strapping older brother; he's a tad jealous. See them in Marvel Cinematic Universe.
Severus Snape is a misanthropic potions teacher with a vindictive streak. See them in Harry Potter Series.
He's an eccentric pirate making it up as he goes along. He's Jack Sparrow, savvy? See them in Pirates of the Caribbean: the Curse of the Black Pearl.
A bookish know-it-all with a bossy streak, Hermione Granger always stands up for what she believes in. See them in Harry Potter Series.